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This book describes the main concepts used to develop and implement chemistry-transport models to calculate the evolution of regional air pollution. Since physico-chemical principles are already widely presented in various works, the perspective chosen for this book concerns the modeling of these processes. As modeling can be a simplification of reality in a particular study framework, we will try to show whether the processes represented are well modeled or not. For each process, we will discuss the simplifying assumptions that have been made, the various possible ways for improvement and the impact of these simplifications on the desired results. General information on pollution is presented, followed by observations, legislation, modeling of meteorology and then chemistry-transport, anthropogenic and natural emissions, depots, validation of calculations, optimization and data assimilation.
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Seitenzahl: 432
Veröffentlichungsjahr: 2024
SCIENCES
Climate and Atmosphere,Field Director – Denis-Didier Rousseau
Atmospheric Physico-Chemistry, Subject Head – Benoit Laurent
Laurent Menut
First published 2024 in Great Britain and the United States by ISTE Ltd and John Wiley & Sons, Inc.
Apart from any fair dealing for the purposes of research or private study, or criticism or review, as permitted under the Copyright, Designs and Patents Act 1988, this publication may only be reproduced, stored or transmitted, in any form or by any means, with the prior permission in writing of the publishers, or in the case of reprographic reproduction in accordance with the terms and licenses issued by the CLA. Enquiries concerning reproduction outside these terms should be sent to the publishers at the under mentioned address:
ISTE Ltd27-37 St George’s RoadLondon SW19 4EUUK
www.iste.co.uk
John Wiley & Sons, Inc.111 River StreetHoboken, NJ 07030USA
www.wiley.com
© ISTE Ltd 2024The rights of Laurent Menut to be identified as the author of this work have been asserted by him in accordance with the Copyright, Designs and Patents Act 1988.
Any opinions, findings, and conclusions or recommendations expressed in this material are those of the author(s), contributor(s) or editor(s) and do not necessarily reflect the views of ISTE Group.
Library of Congress Control Number: 2023942929
British Library Cataloguing-in-Publication DataA CIP record for this book is available from the British LibraryISBN 978-1-78945-102-3
ERC code:PE10 Earth System Science PE10_1 Atmospheric chemistry, atmospheric composition, air pollution
This text introduces the modeling of atmospheric pollution at a regional level. It goes back to the M1 (Masters 1) syllabus put together for the Magisterium at ENS Paris. As the physicochemical principles have already largely been introduced in other texts, the point of view for this book is the modeling of all these processes. Given that modeling is, in reality, a simplification within a particular framework, we will strive to demonstrate whether or not the processes to be represented, such as emission, chemistry and deposits, have been modeled well. There will be a discussion on the simplifying hypothesis used for each model, the ways in which these can be refined and the impact of these simplifications on the desired results. This text cites references that have been chosen for their relevance but also because these articles are free to access online through scientific journals. These references are therefore in italics. When they exist and are OpenAcess, the journal articles will be listed at the beginning of a chapter or a section. A list of all of these articles is given as follows:
Atmospheric pollution, generalities and measurements:
(Monks et al.
2015
)
:
https://acp.copernicus.org/articles/15/8889/2015/
;
(Benedetti et al.
2018
)
:
https://acp.copernicus.org/articles/18/10615/2018/
.
Gaseous chemical and aerosols:
(Stockwell et al.
2012
)
:
https://www.mdpi.com/2073-4433/3/1/1
;
(Carslaw et al.
2010
)
:
https://www.atmos-chem-phys.net/10/1701/2010/
;
(Kanakidou et al.
2005
)
:
https://www.atmos-chem-phys.org/acp/5/1053/
;
(Fuzzi et al.
2015
)
:
https://acp.copernicus.org/articles/15/8217/2015/
.
Emissions:
Anthropic:
(Im et al.
2018
b)
:
https://acp.copernicus.org/articles/18/8929/2018/
.
Biogenic:
(Guenther et al.
2006
)
:
https://acp.copernicus.org/articles/6/3181/2006/
;
(Guenther et al.
2012
)
:
https://gmd.copernicus.org/articles/5/1471/2012/
.
Biomass burning:
(Reid et al.
2005
a)
:
https://acp.copernicus.org/articles/5/799/2005/
;
(Paugam et al.
2016
)
:
http://www.atmos-chem-phys.net/16/907/2016/
.
Mineral aerosols:
(
Schepanski
2018
):
https://www.mdpi.com/2076-3263/8/5/151
.
Volcanoes:
https://acp.copernicus.org/articles/special_issue212.html
.
Lightning:
(Schumann and Huntrieser
2007
)
:
https://www.atmos-chem-phys.net/7/3823/2007/
.
Marine aerosols:
(Gantt and Meskhidze
2013
)
:
https://acp.copernicus.org/articles/13/3979/2013/
.
Pollen:
(Sofiev et al.
2013
a)
:
https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3527742/
.
Deposition:
Dry deposition:
(Pleim and Ran
2011
)
:
https://www.mdpi.com/2073-4433/2/3/271
;
(Vivanco et al.
2018
)
:
https://www.atmos-chem-phys-discuss.net/acp-2018-104/
.
Wet deposition:
(Zhang et al.
2019
)
:
https://doi.org/10.1029/2018JD029051
.
Modeling:
Current models:
(Baklanov et al.
2014
)
:
http://www.atmos-chem-phys.net/14/317/2014/
.
Aerosol models:
(Semeniuk and Dastoor
2020
)
:
https://www.mdpi.com/2073-4433/11/2/156
.
Data assimilation:
(Sandu and Chai
2011
)
:
https://www.mdpi.com/2073-4433/2/3/426
;
(Bocquet et al.
2015
)
:
https://acp.copernicus.org/articles/15/5325/2015/
.
Prediction:
(Marécal et al.
2015
)
:
https://gmd.copernicus.org/articles/8/2777/2015/
.
Coupling:
(Zhang
2008
)
:
https://acp.copernicus.org/articles/8/2895/2008/
;
(Baklanov et al.
2014
)
:
http://www.atmos-chem-phys.net/14/317/2014/
.
There are other journal articles, but behind a paywall. These references are indicated in bold. They are cited directly within the relevant chapters. This text is also based on other books, including (Jacob 1999), (Delmas et al. 2005), (Pielke 2013), (Jacobson 1999), (Stensrud 2011), (Shao 2004), (Seinfeld and Pandis 2006) and (Stull 1988).
For each chapter, the key points are summarized in gray boxes like this one.
November 2023